Affiliations 

  • 1 Institute of Advanced Technology, Universiti Putra Malaysia, UPM Serdang 43400, Selangor, Malaysia. [email protected]
  • 2 Chemical Engineering Department, Khalifa University, Abu Dhabi 127788, United Arab Emirates
  • 3 School of Chemistry and Environment, Faculty of Applied Sciences, Universiti Teknologi MARA, Shah Alam 40450, Selangor, Malaysia
  • 4 National Centre of Excellence in Physical Chemistry, University of Peshawar, Peshawar 25120, Pakistan
  • 5 Department of Chemistry, University of Agriculture Faisalabad, Faisalabad 38000, Pakistan
  • 6 Department of Chemical and Environmental Engineering, Engineering Faculty, Universiti Putra Malaysia, UPM Serdang 43400, Selangor, Malaysia
Materials (Basel), 2019 Jul 18;12(14).
PMID: 31323732 DOI: 10.3390/ma12142293

Abstract

The main purpose of this manuscript is to report the new usage of tea waste (TW) as a catalyst for efficient conversion of palm fatty acid distillate (PFAD) to biodiesel. In this work, we investigate the potential of tea waste char as a catalyst for biodiesel production before and after sulfonation. The activated sulfonated tea waste char catalyst was characterized using Fourier transform infrared spectroscopy (FTIR), thermogravimetric analysis (TGA), X-ray diffractometry (XRD), elemental composition (CHNS), nitrogen adsorption-desorption using Brunauer-Emmett-Teller (BET) and ammonia-temperature-programmed desorption (NH3-TPD). The activated tea waste char catalyst shows higher acid density of 31 μmol g-1 as compared to tea waste char of 16 μmol g-1 and higher surface area of 122 m2/g. The optimum fatty acid conversion conditions were found that 4 wt % of catalyst loading with 9:1 of methanol:PFAD for 90 min of reaction time at 65 °C gives 97% free fatty acid (FFA) conversion. In conclusion, the sulfonated tea waste (STW) catalyst showed an impressive catalytic activity towards the esterification of PFAD at optimum reaction conditions with significant recyclability in five successive cycles without any reactivation step.

* Title and MeSH Headings from MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine.