Affiliations 

  • 1 Department of Petroleum and Mining Engineering, Jashore University of Science and Technology, Jashore, 7408, Bangladesh; Clean Energy and CO(2) Capture Lab, Jashore University of Science and Technology, Jashore, 7408, Bangladesh. Electronic address: [email protected]
  • 2 Faculty Science and Natural Resources, Universiti Malaysia Sabah, Jalan UMS, 88400, Kota Kinabalu, Sabah, Malaysia
  • 3 Department of Petroleum and Mining Engineering, Jashore University of Science and Technology, Jashore, 7408, Bangladesh; Clean Energy and CO(2) Capture Lab, Jashore University of Science and Technology, Jashore, 7408, Bangladesh
  • 4 Department of Textile Engineering, Dhaka University of Engineering & Technology, Gzipur, 1707, Bangladesh
  • 5 School of Chemistry and Environment, Faculty of Applied Sciences, Universiti Teknologi MARA, 40450, Shah Alam, Selangor, Malaysia
  • 6 Center of Excellence for Green Energy and Environmental Nanomaterials (CE@GrEEN), Nguyen Tat Thanh University, 300A Nguyen Tat Thanh, District 4, Ho Chi Minh City, 755414, Viet Nam
  • 7 Chemical and Environmental Engineering Department, Faculty of Engineering, Universiti Putra Malaysia, 43400, UPM, Serdang, Selangor, Malaysia
  • 8 Asia Arsenic Network, Arsenic Center, Benapole Road, Krishnobati, Pulerhat, Jessore, Bangladesh
Chemosphere, 2021 Jun;272:129653.
PMID: 33486455 DOI: 10.1016/j.chemosphere.2021.129653

Abstract

The contamination of groundwater by arsenic (As) in Bangladesh is the biggest impairing of a population, with a large number of peoples affected. Specifically, groundwater of Gangetic Delta is alarmingly contaminated with arsenic. Similar, perilous circumstances exist in many other countries and consequently, there is a dire need to develop cost-effective decentralized filtration unit utilizing low-cost adsorbents for eliminating arsenic from water. Morphological synthesis of carbon with unique spherical, nanorod, and massive nanostructures were achieved by solvothermal method. Owing to their intrinsic adsorption properties and different nanostructures, these nanostructures were employed as adsorption of arsenic in aqueous solution, with the purpose to better understanding the morphological effect in adsorption. It clearly demonstrated that carbon with nanorods morphology exhibited an excellent adsorption activity of arsenite (about 82%) at pH 3, remarkably superior to the two with solid sphere and massive microstructures, because of its larger specific surface area, enhanced acid strength and improved adsorption capacity. Furthermore, we discovered that iron hydroxide radicals and energy-induced contact point formation in nanorods are the responsible for the high adsorption of As in aqueous solution. Thus, our work provides insides into the microstructure-dependent capability of different carbon for As adsorption applications.

* Title and MeSH Headings from MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine.